Over the last few years, there has been a convergence between the fields of ultrafast science, nonlinear optics, optical frequency metrology, and precision laser spectroscopy. These fields have been developing largely independently since the birth of the laser, reaching remarkable levels of performance. On the ultrafast frontier, pulses of only a few cycles long have been produced, while in optical spectroscopy, the precision and resolution have reached one part in Although these two achievements appear to be completely disconnected, advances in nonlinear optics provided the essential link between them. The resulting convergence has enabled unprecedented advances in the control of the electric field of the pulses produced by femtosecond mode-locked lasers. The corresponding spectrum consists of a comb of sharp spectral lines with well-defined frequencies. These new techniques and capabilities are generally known as “femtosecond comb technology. ” They have had dramatic impact on the diverse fields of precision measurement and extreme nonlinear optical physics. The historical background for these developments is provided in the Foreword by two of the pioneers of laser spectroscopy, John Hall and Theodor Hänsch. Indeed the developments described in this book were foreshadowed by Hänsch’s early work in the 1970s when he used picosecond pulses to demonstrate the connection between the time and frequency domains in laser spectroscopy. This work complemented the advances in precision laser stabilization developed by Hall.

Ultrashort Laser Pulse Phenomena, Second Edition serves as an introduction to the phenomena of ultra short laser pulses and describes how this technology can be used to examine problems in areas such as electromagnetism, optics, and quantum mechanics. Ultrashort Laser Pulse Phenomena combines theoretical backgrounds and experimental techniques and will serve as a manual on designing and constructing femtosecond ("faster than electronics") systems or experiments from scratch. Beyond the simple optical system, the various sources of ultrashort pulses are presented, again with emphasis on the basic concepts and how they apply to the design of particular sources (dye lasers, solid state lasers, semiconductor lasers, fiber lasers, and sources based on frequency conversion). - Provides an easy to follow guide through "faster than electronics" probing and detection methods - THE manual on designing and constructing femtosecond systems and experiments - Discusses essential technology for applications in micro-machining, femtochemistry, and medical imaging

Energy-efficient Tbit/s optical interconnects are key elements for future communication systems. Three novel optical frequency comb sources are investigated, which have the potential of being integrated in chip-scale Tbit/s transmitters. Such frequency combs provide a large number of carriers. The equidistance of the comb lines helps to minimize spectral guard bands. For each type of comb source, coherent data transmission experiments show the potential for Tbit/s data transmission rates.

To keep up with the ever-increasing data transmission speed needs, data center interconnects are scaling up to provide multi-Tbit/s connectivity. These links require a high number of WDM channels, while the associated transceivers should be compact and energy efficient. Scaling the number of channels, however, is still limited by the lack of adequate optical sources. In this book, we investigate novel chip-scale frequency comb generators as multi-wavelength light sources for Tbit/s WDM links.

Advances in Quantum Chemistry presents surveys of current topics in this rapidly developing field that has emerged at the cross section of the historically established areas of mathematics, physics, chemistry, and biology. It features detailed reviews written by leading international researchers. This series provides a one-stop resource for following progress in this interdisciplinary area. - Publishes articles, invited reviews and proceedings of major international conferences and workshops - Written by leading international researchers in quantum and theoretical chemistry - Highlights important interdisciplinary developments

This book introduces readers to the development of a new generation of high pulse-repetition frequency instruments for multi-dimensional attosecond-resolution photoelectron spectroscopy (attosecond PES). It investigates the power scaling of femtosecond enhancement cavities for efficient intracavity high-harmonics generation (HHG). Further, it derives and verifies advanced resonator designs that feature large illuminated spots on all mirrors, which mitigate both intensity- and thermally-induced enhancement limitations. The dynamics of a high-finesse, passive resonator in the presence of a highly nonlinear optical process such as HHG are quantitatively investigated, both theoretically and experimentally. These investigations are instrumental in achieving the holistic optimization of the XUV source reported on here, which for the first time reached intracavity HHG conversion efficiencies comparable to those achieved in single-pass setups with a similar gas target. Coupling out the XUV beam from the enhancement cavity by purely geometric means, employing both the fundamental and higher-order transverse Gaussian modes, is studied. This offers the advantages of robustness, low distortion to the participating pulses, and photon-energy scalability. Last but not least, the author provides a range of proof-of-principle attosecond angle-resolved PES experiments. The book gives an outlook on the possible future development of cavity-enhanced HHG and an extensive discussion on the generation of isolated XUV attosecond pulses via intracavity wavefront rotation.

This comprehensive handbook gives a fully updated guide to lasers and laser systems, including the complete range of their technical applications. The first volume outlines the fundamental components of lasers, their properties and working principles. The second volume gives exhaustive coverage of all major categories of lasers, from solid-state and semiconductor diode to fiber, waveguide, gas, chemical, and dye lasers. The third volume covers modern applications in engineering and technology, including all new and updated case studies spanning telecommunications and data storage to medicine, optical measurement, defense and security, nanomaterials processing and characterization.

Optical frequency combs (OFC) have revolutionized various applications in applied and fundamental sciences that rely on the determination of absolute optical frequencies and frequency differences. The latter requires only stabilization of the spectral distance between the individual comb lines of the OFC, allowing to tailor and reduce system complexity of the OFC generator (OFCG). One such application is the quantum test of the universality of free fall within the QUANTUS experimental series. Within the test, the rate of free fall of two atomic species, Rb and K, in micro-gravity will be compared. The aim of this thesis was the development of a highly compact, robust, and space-suitable diode laser-based OFCG with a mode-locked optical spectrum in the wavelength range around 780 nm. A diode laser-based OFCG was developed, which exceeds the requirements with a spectral bandwidth > 16 nm at 20 dBc, a comb line optical power > 650 nW (at 20 dBc), a pulse repetition rate of 3.4 GHz, and an RF linewidth of the free-running pulse repetition rate < 10 kHz. To realize a proof-of-concept demonstrator module, the diode laser-based OFCG was hybrid-integrated into a space-suitable technology platform that has been developed for future QUANTUS experiments. Proof of sufficient RF stability of the OFCG was provided by stabilizing the pulse repetition rate to an external RF reference. This resulted in a stabilized pulse repetition rate with an RF linewidth smaller than 1.4 Hz (resolution limited), thus exceeding the requirement. The developed diode laser-based OFCG represents an important step towards an improved comparison of the rate of free fall of Rb and K quantum gases within the QUANTUS experiments in micro-gravity.

This thesis presents first successful experiments to carrier-envelope-phase stabilize a high-power mode-locked thin-disk oscillator and to compress the pulses emitted from this laser to durations of only a few-optical cycles. Moreover, the monograph introduces several methods to achieve power-scalability of compression and stabilization techniques. All experimental approaches are compared in detail and may serve as a guideline for developing high-power waveform controlled, few-cycle light sources which offer tremendous potential to exploit extreme nonlinear optical effects at unprecedentedly high repetition rates and to establish table-top infrared light sources with a unique combination of brilliance and bandwidth. As an example, the realization of a multi-Watt, multi-octave spanning, mid-infrared femtosecond source is described. The thesis starts with a basic introduction to the field of ultrafast laser oscillators. It subsequently presents additional details of previously published research results and establishes a connection between them. It therefore addresses both newcomers to, and experts in the field of high-power ultrafast laser development.

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